There is a huge thread on Epoxy Granites that you can look into. Some people have used concretes and even sand.
There is a very good PDF that floats around the net called: "The Principles of Rapid Machine Design" by Eberhard Bamberg that is well worth a read. It has more information than you might want though, but it USA very good read none the less.
I haven't actually filled anything myself so I can't suggest anything based on experience. What I would or may do in the future is go the epoxy fill route. That is epoxy mixed with aggregate to make a plastic concrete.
As to the gap fillers I wouldn't waste my time! I've used many cans of that stuff to insulate my house, as such I have a hard time believing it could do a lot for you. Maybe others could chime in here with actual experience and objective tests. While I'm not one to throw the "add mass" dogma around putting the right materials in the right places can be very useful. This material adds no mass to speak of but could possibly change resonance.